Wood waste-based functionalized natural hydrochar for the effective removal of Ce(III) ions from aqueous solution

dc.creatordos Reis, Glaydson S.
dc.creatorSchnorr, Carlos Eduardo
dc.creatorDotto, Guilherme Luiz
dc.creatorVieillard, Julien
dc.creatorNetto, Matias S.
dc.creatorSilva Oliveira, Luis Felipe
dc.creatorDe Brum, Irineu A. S.
dc.creatorThyrel, Mikael
dc.creatorLima, Éder C.
dc.creatorLassi, Ulla
dc.date2023-09-18T16:17:45Z
dc.date2024
dc.date2023-09-18T16:17:45Z
dc.date2023
dc.date.accessioned2023-10-03T19:40:20Z
dc.date.available2023-10-03T19:40:20Z
dc.identifierdos Reis, G.S., Schnorr, C.E., Dotto, G.L. et al. Wood waste-based functionalized natural hydrochar for the effective removal of Ce(III) ions from aqueous solution. Environ Sci Pollut Res 30, 64067–64077 (2023). https://doi.org/10.1007/s11356-023-26921-6
dc.identifier0944-1344
dc.identifierhttps://hdl.handle.net/11323/10494
dc.identifier10.1007/s11356-023-26921-6
dc.identifier1614-7499
dc.identifierCorporación Universidad de la Costa
dc.identifierREDICUC - Repositorio CUC
dc.identifierhttps://repositorio.cuc.edu.co/
dc.identifier.urihttps://repositorioslatinoamericanos.uchile.cl/handle/2250/9171262
dc.descriptionIn this study, a sustainable and easily prepared hydrochar from wood waste was studied to adsorb and recover the rare earth element cerium (Ce(III)) from an aqueous solution. The results revealed that the hydrochar contains several surface functional groups (e.g., C–O, C = O, OH, COOH), which largely influenced its adsorption capacity. The effect of pH strongly influenced the Ce(III) removal, achieving its maximum removal efficiency at pH 6.0 and very low adsorption capacity under an acidic solution. The hydrochar proved to be highly efficient in Ce(III) adsorption reaching a maximum adsorption capacity of 327.9 mg g−1 at 298 K. The kinetic and equilibrium process were better fitted by the general order and Liu isotherm model, respectively. Possible mechanisms of Ce(III) adsorption on the hydrochar structure could be explained by electrostatic interactions and chelation between surface functional groups and the Ce(III). Furthermore, the hydrochar exhibited an excellent regeneration capacity upon using 1 mol L−1 of sulfuric acid (H2SO4) as eluent, and it was reused for three cycles without losing its adsorption performance. This research proposes a sustainable approach for developing an efficient adsorbent with excellent physicochemical and adsorption properties for Ce(III) removal.
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dc.languageeng
dc.publisherSpringer Science + Business Media
dc.publisherGermany
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dc.rights© 2023 Springer Nature
dc.rightsAtribución 4.0 Internacional (CC BY 4.0)
dc.rightshttps://creativecommons.org/licenses/by/4.0/
dc.rightsinfo:eu-repo/semantics/embargoedAccess
dc.rightshttp://purl.org/coar/access_right/c_f1cf
dc.sourcehttps://link.springer.com/article/10.1007/s11356-023-26921-6
dc.subjectWood waste
dc.subjectHydrochar
dc.subjectSustainable material
dc.subjectRare earth element
dc.subjectCerium
dc.subjectAdsorption
dc.subjectRecovery
dc.titleWood waste-based functionalized natural hydrochar for the effective removal of Ce(III) ions from aqueous solution
dc.typeArtículo de revista
dc.typehttp://purl.org/coar/resource_type/c_2df8fbb1
dc.typeText
dc.typeinfo:eu-repo/semantics/article
dc.typehttp://purl.org/redcol/resource_type/ART
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