Application of araçá fruit husks (Psidium cattleianum) in the preparation of activated carbon with FeCl3 for atrazine herbicide adsorption

dc.creatorLazarotto, Joseane
dc.creatorDA BOIT MARTINELLO, KATIA
dc.creatorgeorgin, jordana
dc.creatorFranco, Dison S.P.
dc.creatorNetto, Matias S.
dc.creatorPiccilli, Daniel G.A.
dc.creatorSilva, Luis F.O.
dc.creatorLima, Eder Claudio
dc.creatorDotto, Guilherme Luiz
dc.date2022-06-14T16:19:57Z
dc.date2024-04
dc.date2022-06-14T16:19:57Z
dc.date2022-04
dc.date.accessioned2023-10-03T19:11:09Z
dc.date.available2023-10-03T19:11:09Z
dc.identifierJoseane S. Lazarotto, Kátia da Boit Martinello, Jordana Georgin, Dison S.P. Franco, Matias S. Netto, Daniel G.A. Piccilli, Luis F.O. Silva, Eder C. Lima, Guilherme L. Dotto, Application of araçá fruit husks (Psidium cattleianum) in the reparation of activated carbon with FeCl3 for atrazine herbicide adsorption, Chemical Engineering Research and Design, Volume 180, 2022, Pages 67-78, ISSN 0263-8762, https://doi.org/10.1016/j.cherd.2022.01.044.
dc.identifier0263-8762
dc.identifierhttps://hdl.handle.net/11323/9254
dc.identifier10.1016/j.cherd.2022.01.044.
dc.identifier17443563
dc.identifierCorporación Universidad de la Costa
dc.identifierREDICUC - Repositorio CUC
dc.identifierhttps://repositorio.cuc.edu.co/
dc.identifier.urihttps://repositorioslatinoamericanos.uchile.cl/handle/2250/9168643
dc.descriptionThe residual husks of the edible fruits of Psidium cattleianum were carbonized with FeCl3 as an activating agent and used as an adsorbent to remove the toxic herbicide. After the carbonization step, changes in the material’s structure were found. Activated carbon showed characteristics of microporous materials with a pore volume of 0.280 cm3 g−1 and surface area of 431 m2 g−1. Micrographs revealed the emergence of new cavities with a uniform and circular shape. The FTIR spectra showed the disappearance of some bands, remaining bands belonging to functional groups containing carbon, oxygen, and hydrogen. The XRD patterns confirmed the amorphous structure of the material even after the carbonization step, composed of amorphous graphitic carbon. EDS analysis showed that the carbon percentage increased and the oxygen decreased after the carbonization. The experiments were performed at neutral pH using 1 g L−1 of adsorbent. In equilibrium isotherms, the temperature played a considerable role in the adsorption capacity, increasing from 26.39 mg g−1 to 35.67 mg g−1 when the temperature varied from 298 to 328 K. The Liu isotherms were the ones that best fit the isotherm data. The changes in the adsorption enthalpy were endothermic (ΔH° 129.5 kJ mol−1). The general order kinetic model was the most adequate for kinetic data, presenting the lowest values of the Bayesian Information Criterion. Thus, activated carbon developed from the residues of the “araça” fruit showed promise in removing atrazine from aqueous solutions, with the great advantage of its high efficiency under neutral pH solutions and mild temperatures.
dc.format12 paginas
dc.formatapplication/pdf
dc.formatapplication/pdf
dc.languageeng
dc.publisherInstitution of Chemical Engineers
dc.publisherUnited Kingdom
dc.relationChemical Engineering Research and Design
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dc.rightsAtribución-NoComercial-SinDerivadas 4.0 Internacional (CC BY-NC-ND 4.0)
dc.rights© 2022 Institution of Chemical Engineers. Published by Elsevier Ltd. All rights reserved.
dc.rightshttps://creativecommons.org/licenses/by-nc-nd/4.0/
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dc.rightshttp://purl.org/coar/access_right/c_f1cf
dc.sourcehttps://www.sciencedirect.com/science/article/pii/S0263876222000521
dc.subjectAdsorption
dc.subjectAtrazine
dc.subjectActivated carbon
dc.subjectAdsorption thermodynamics
dc.subjectBiomass-based adsorbent
dc.titleApplication of araçá fruit husks (Psidium cattleianum) in the preparation of activated carbon with FeCl3 for atrazine herbicide adsorption
dc.typeArtículo de revista
dc.typehttp://purl.org/coar/resource_type/c_6501
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dc.typeinfo:eu-repo/semantics/article
dc.typeinfo:eu-repo/semantics/publishedVersion
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