Transfer of radon and parent nuclides U-238 and U-234 from soils of the Mendip Hills area, England, to the water phase

dc.contributorUniversidade Estadual Paulista (UNESP)
dc.creatorBonotto, Daniel Marcos
dc.creatorAndrews, J. N.
dc.date2014-05-20T15:20:59Z
dc.date2016-10-25T17:54:12Z
dc.date2014-05-20T15:20:59Z
dc.date2016-10-25T17:54:12Z
dc.date1999-07-01
dc.date.accessioned2017-04-05T23:28:38Z
dc.date.available2017-04-05T23:28:38Z
dc.identifierJournal of Geochemical Exploration. Amsterdam: Elsevier B.V., v. 66, n. 1-2, p. 255-268, 1999.
dc.identifier0375-6742
dc.identifierhttp://hdl.handle.net/11449/32171
dc.identifierhttp://acervodigital.unesp.br/handle/11449/32171
dc.identifier10.1016/S0375-6742(99)00016-3
dc.identifierWOS:000081683100023
dc.identifierhttp://dx.doi.org/10.1016/S0375-6742(99)00016-3
dc.identifier.urihttp://repositorioslatinoamericanos.uchile.cl/handle/2250/876559
dc.descriptionLaboratory time scale experiments were conducted on soils from the Mendip Hills area, England, with the purpose of evaluating the release of Rn-222 and their parent nuclides U-238 and U-234 to the water phase and to determine the influence of parameters that can affect the geochemical behaviour of these nuclides in natural systems. The specific surface area of the samples ranged from 43.8 to 52.5 cm(2) g(-1), where the particle size for all soil horizons is lognormally distributed, with modal values of the particle radius undersize ranging from 107 up to 203 mu m. The values for the released radon were between 26 and 194 pCi, which allowed to estimate emanation coefficients for these materials between 0.1 and 0.2, within the context of other values reported elsewhere. Soils derived from Carboniferous limestone and characterized by higher pH, exchangeable calcium, and the presence of U, but with a lower U-231/U-238 activity ratio, yielded the highest values for released Rn; however, this trend was not observed for dissolved U and its respective U-234/U-238 activity ratio, when considering the less aggressive etchant. Uranium is mobilized from rock matrix to A and B horizons in the analysed soil profiles, where its enrichment is about 10 times higher in soils derived from Carboniferous limestone. These data also permitted an evaluation of a theoretical model for the generation of Rn in soils and its transfer to water, in order to interpret the radioactivity due to this gas in groundwaters from the Mendip Hills district, England. (C) 1999 Elsevier B.V. B.V. All lights reserved.
dc.languageeng
dc.publisherElsevier B.V.
dc.relationJournal of Geochemical Exploration
dc.rightsinfo:eu-repo/semantics/closedAccess
dc.subjectradon
dc.subjecturanium
dc.subjectgeochemical behaviour
dc.subjectmodel
dc.subjectsoils
dc.subjectwater
dc.subjectEngland
dc.titleTransfer of radon and parent nuclides U-238 and U-234 from soils of the Mendip Hills area, England, to the water phase
dc.typeOtro


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