dc.creatorBrinks, Daan
dc.creatorHildner, Richard
dc.creatorStefani, Fernando Daniel
dc.creatorVan Hulst, Niek F.
dc.date.accessioned2019-01-29T21:27:42Z
dc.date.accessioned2022-10-15T13:38:13Z
dc.date.available2019-01-29T21:27:42Z
dc.date.available2022-10-15T13:38:13Z
dc.date.created2019-01-29T21:27:42Z
dc.date.issued2011-12
dc.identifierBrinks, Daan; Hildner, Richard; Stefani, Fernando Daniel; Van Hulst, Niek F.; Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments; Optical Society of America; Optics Express; 19; 27; 12-2011; 26486-26499
dc.identifier1094-4087
dc.identifierhttp://hdl.handle.net/11336/68943
dc.identifierCONICET Digital
dc.identifierCONICET
dc.identifier.urihttps://repositorioslatinoamericanos.uchile.cl/handle/2250/4392199
dc.description.abstractDiffraction of finite sized laser beams imposes a limit on the control that can be exerted over ultrafast pulses. This limit manifests as spatio-temporal coupling induced in standard implementations of pulse shaping schemes. We demonstrate the influence this has on coherent control experiments that depend on finite excitation, sample, and detection volumes. Based on solutions used in pulse stretching experiments, we introduce a double-pass scheme that reduces the errors produced through spatio-temporal coupling by at least one order of magnitude. Finally, employing single molecules as nanoscale probes, we prove that such a double pass scheme is capable of artifact-free pulse shaping at dimensions two orders of magnitude smaller than the diffraction limit.
dc.languageeng
dc.publisherOptical Society of America
dc.relationinfo:eu-repo/semantics/altIdentifier/url/https://www.osapublishing.org/oe/abstract.cfm?uri=oe-19-27-26486
dc.relationinfo:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1364/OE.19.026486
dc.rightshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.rightsinfo:eu-repo/semantics/openAccess
dc.subjectultrafast spectroscopy
dc.subjectpulse shaper
dc.titleBeating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
dc.typeinfo:eu-repo/semantics/article
dc.typeinfo:ar-repo/semantics/artículo
dc.typeinfo:eu-repo/semantics/publishedVersion


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