dc.contributorAlexey Krasavin
dc.contributorRuth Webster
dc.contributorPAULINA SEGOVIA OLVERA
dc.contributorAnatoly Zayats
dc.contributorDavid Richards
dc.creatorJia Li
dc.date2016
dc.date.accessioned2022-10-12T19:37:01Z
dc.date.available2022-10-12T19:37:01Z
dc.identifierhttp://cicese.repositorioinstitucional.mx/jspui/handle/1007/1760
dc.identifier.urihttps://repositorioslatinoamericanos.uchile.cl/handle/2250/4118503
dc.description"We explore the spectral dependence of fluorescence enhancement and the associated lifetime modification of fluorescent molecules coupled to single metal nanoparticles. Fluorescence lifetime imaging microscopy and single-particle dark-field spectroscopy are combined to correlate the dependence of fluorescence lifetime reduction on the spectral overlap between the fluorescence emission and the localised surface plasmon (LSP) spectra of individual gold nanoparticles. A maximum lifetime reduction is observed when the fluorescence and LSP resonances coincide, with good agreement provided by numerical simulations. The explicit comparison between experiment and simulation, that we obtain, offers an insight into the spectral engineering of LSP mediated fluorescence and may lead to optimized application in sensing and biomedicine."
dc.formatapplication/pdf
dc.languageeng
dc.publisherNature Publishing Group
dc.relationinfo:eu-repo/semantics/altIdentifier/DOI/http://dx.doi.org/10.1038/srep21349
dc.relationcitation:Li,J.,Krasavin,A.V.,Webster,L.,Segovia,P.,Zayats,A.V.,Richards,D.2016.Spectral variation of fluorescence lifetime near single metal nanoparticles.Scientific Reports,6,1-8.doi:10.1038/srep21349
dc.rightsinfo:eu-repo/semantics/openAccess
dc.rightshttp://creativecommons.org/licenses/by-nc-nd/4.0
dc.sourceScientific Reports, Vol. 6, Págs. 1-8
dc.subjectinfo:eu-repo/classification/Autor/Fluorescence spectroscopy, Nanoparticles, Nanophotonics and plasmonics
dc.subjectinfo:eu-repo/classification/cti/1
dc.subjectinfo:eu-repo/classification/cti/22
dc.subjectinfo:eu-repo/classification/cti/2209
dc.titleSpectral variation of fluorescence lifetime near single metal nanoparticles
dc.typeinfo:eu-repo/semantics/article
dc.typeinfo:eu-repo/semantics/publishedVersion


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