dc.date2015
dc.date2016-06-03T20:14:07Z
dc.date2016-06-03T20:14:07Z
dc.date.accessioned2018-03-29T01:33:04Z
dc.date.available2018-03-29T01:33:04Z
dc.identifier
dc.identifierPhysical Review B - Condensed Matter And Materials Physics. American Physical Society, v. 92, n. 8, p. , 2015.
dc.identifier10980121
dc.identifier10.1103/PhysRevB.92.081114
dc.identifierhttp://www.scopus.com/inward/record.url?eid=2-s2.0-84941116612&partnerID=40&md5=e13bd1271e85a663a12024367056a904
dc.identifierhttp://repositorio.unicamp.br/jspui/handle/REPOSIP/238175
dc.identifier2-s2.0-84941116612
dc.identifier.urihttp://repositorioslatinoamericanos.uchile.cl/handle/2250/1304836
dc.descriptionIn a combined experimental and theoretical study, we investigate the properties of Sr2Ir1-xRhxO4. From the branching ratios of the L-edge isotropic x-ray absorption spectra, we determine that the spin-orbit coupling is remarkably independent of x for both iridium and rhodium sites. DFT+U calculations show that the doping is close to isoelectronic and introduces impurity bands of predominantly rhodium character close to the lower Hubbard band. Overlap of these two bands leads to metallic behavior. Since the low-energy states for x<0.5 have predominantly jeff=12 character, we suggest that the electronic properties of this material can be described by an inhomogeneous Hubbard model, where the on-site energies change due to local variations in the spin-orbit interaction strength combined with additional changes in binding energy. © 2015 American Physical Society.
dc.description92
dc.description8
dc.description
dc.description
dc.description2014R1A1A2057202, National Research Foundation
dc.descriptionDMR-1265162, NSF, National Research Foundation
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dc.description
dc.description
dc.languageen
dc.publisherAmerican Physical Society
dc.relationPhysical Review B - Condensed Matter and Materials Physics
dc.rightsaberto
dc.sourceScopus
dc.titleSr2ir1-xrhx O4(x < 0.5): An Inhomogeneous Jeff= 12 Hubbard System
dc.typeArtículos de revistas


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