dc.creatorLisi L.
dc.creatorMarchese L.
dc.creatorPastore H.O.
dc.creatorFrache A.
dc.creatorRuoppolo G.
dc.creatorRusso G.
dc.date2003
dc.date2015-06-30T17:30:03Z
dc.date2015-11-26T14:08:21Z
dc.date2015-06-30T17:30:03Z
dc.date2015-11-26T14:08:21Z
dc.date.accessioned2018-03-28T21:08:56Z
dc.date.available2018-03-28T21:08:56Z
dc.identifier
dc.identifierTopics In Catalysis. , v. 22, n. 01/02/15, p. 95 - 99, 2003.
dc.identifier10225528
dc.identifier10.1023/A:1021424030847
dc.identifierhttp://www.scopus.com/inward/record.url?eid=2-s2.0-0242527341&partnerID=40&md5=5f4a4f600e830a031c7e76473d17c376
dc.identifierhttp://www.repositorio.unicamp.br/handle/REPOSIP/102320
dc.identifierhttp://repositorio.unicamp.br/jspui/handle/REPOSIP/102320
dc.identifier2-s2.0-0242527341
dc.identifier.urihttp://repositorioslatinoamericanos.uchile.cl/handle/2250/1240982
dc.descriptionAcid silicoaluminophosphate SAPO-34 catalysts with a chabasite-related structure were evaluated for the oxidative dehydrogenation of ethane at 550°-700°C, achieving very interesting catalytic performances (about 70% C2H4 selectivity at 45% ethane conversion), which were related to both Lewis and Brønsted acid sites. Ethylene, CO, and CO2 were detected in all catalytic tests. Traces of methane were formed only at higher conversions, which makes SAPO-34-based catalysts quite distinct from other zeolites. All acid sites were involved in both ethane activation and ethylene formation in contrast to the behavior of ZSM-5, which was more active and selective when alkali metal ions or transition metal ions were present.
dc.description22
dc.description01/02/15
dc.description95
dc.description99
dc.descriptionCavani, F., Trifirò, F., (1995) Catal. Today, 24, p. 307
dc.descriptionConway, S.J., Wang, D.J., Lunsford, J.H., (1991) Appl. Catal. A: General, 79, pp. L1
dc.descriptionBaerns, M., Buyevskaya, O., (1998) Catal. Today, 45, p. 13
dc.descriptionKennedy, E.M., Cant, N.W., (1992) Appl. Catal. A: General, 87, p. 171
dc.descriptionChourdary, V.R., Rane, V.H., (1992) J. Catal., 135, p. 310
dc.descriptionBordoni, S., Castellani, F., Cavani, F., Trifirò, F., Kulkarni, M.P., (1994) New Developments in Selective Oxidation II, p. 93. , eds. V. Cortés Corberan and S. Vic Bellon (Elsevier, Amsterdam)
dc.descriptionCiambelli, P., Lisi, L., Pirone, R., Ruoppolo, G., Russo, G., (2000) Catal. Today, 61, p. 317
dc.descriptionBanãres, M.A., (1999) Catal. Today, 51, p. 319
dc.descriptionChang, Y.-F., Somorjai, G., Heinemann, H., (1993) Appl. Catal. A: General, 96, p. 305
dc.descriptionChang, Y.-F., Somorjai, G., Heinemann, H., (1995) J. Catal., 154, p. 24
dc.descriptionKubacka, A., Wloch, E., Sulikowski, B., Valenzuela, R.X., Cortés Corberan, V., (2000) Catal. Today, 61, p. 343
dc.descriptionArends, I.W.C.E., Sheldon, R.A., Wallau, M., Schuchardt, U., (1997) Angew. Chem. Int. Ed. Engl., 36, p. 1144
dc.descriptionHuff, M., Schmidt, L.D., (1993) J. Phys. Chem., 97, p. 11815
dc.descriptionSmith, L., Marchese, L., Cheetham, A.K., Thomas, J.M., Wright, P.A., Chen, J., Morris, R.E., (1996) Science, 271, p. 799
dc.descriptionSmith, L., Cheetham, A.K., Marchese, L., Gianotti, E., Thomas, J.M., Wright, P.A., Chen, J., (1996) Catal. Lett., 41, p. 13
dc.descriptionChen, J., Wright, P.A., Thomas, J.M., Natarajan, S., Marchese, L., Bradley, S.M., Sankar, G., Lok, C.M., (1994) J. Phys. Chem., 98, p. 10216
dc.descriptionStöcher, M., (1999) Micropor. Mesopor. Mater., 29, p. 348
dc.descriptionBriend, M., Vomscheid, R., Peltre, M.J., Man, P.P., Barthomeuf, D., (1995) J. Phys. Chem., 99, p. 8270
dc.descriptionMarchese, L., Frache, A., Gianotti, E., Martra, G., Causà, M., Coluccia, S., (1999) Micropor. Mesopor. Mater., 145, p. 30
dc.descriptionMarchese, L., Frache, A., Gatti, G., Coluccia, S., Lisi, L., Ruoppolo, G., Russo, G., Pastore, H.O., J. Catal., , (in press)
dc.descriptionPopova, M., Minchev, Ch., Knazirev, V., (1998) Appl. Catal. A, 169, p. 227
dc.descriptionParlitz, B., Schreier, E., Zubowa, H.L., Eckelt, R., Lieske, E., Lischke, G., Fricke, R., (1995) J. Catal., 155, p. 11
dc.descriptionCatana, G., Baetens, D., Mommaerts, T., Schoonheydt, R.A., Weckhuysen, B.M., (2001) J. Phys, Chem. B, 105, p. 4904
dc.descriptionWoolery, G.L., Kuehl, G.H., Timken, H.C., Chester, A.W., Vartuli, J.C., (1997) Zeolites, 19, p. 288
dc.descriptionBen-Zu, W., Kuangtse, H., (1991) Appl. Catal., 73, p. 113
dc.descriptionConcepcion, P., Corma, A., Lopes Nieto, J.M., Perez-Pariente, J., (1996) Appl. Catal. A: General, 143, p. 17
dc.languageen
dc.publisher
dc.relationTopics in Catalysis
dc.rightsfechado
dc.sourceScopus
dc.titleEvaluating The Catalytic Performances Of Sapo-34 Catalysts For The Oxidative Dehydrogenation Of Ethane
dc.typeArtículos de revistas


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